1 Introduction In the past decade, perovskite solar cells (PSC) evolved into one of the most promising photovoltaic materials, with steadily rising power conversion efficiencies (PCE) now over 26% in the leading examples.[1] The outstanding and promising opto-electronic properties of perovskites, such as a tunable bandgap, high absorption coefficient, and long charge carrier lifetime have enabled this rapid success.[2-6] Nonetheless, organometal halide perovskites suffer from insufficient...