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Topochemical Synthesis of Single-Crystalline Hydrogen-Bonded Cross-Linked Organic Frameworks and Their Guest-Induced Elastic Expansion

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By Russell Hughes, Richard J. Staples, Xuanfeng Jiang, Xunzhe Cui
| American Chemical Society
Covalently linked single-crystalline porous organic materials are highly desired for structure–property analysis; however, periodically polymerizing organic entities into high dimensional networks is challenging. Here, we report a series of topologically divergent single-crystalline hydrogen-bonded cross-linked organic frameworks (HCOFs) with visible guest-induced elastic expansions, which mutually integrate high structural order and high flexibility into one framework.
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