Yin-Hung Lai

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Download Hi-Res ImageDownload to MS-PowerPointCite This:Energy Fuels 2020, XXXX, XXX Jana L. van den Berg Jana L. van den Berg Department of Chemistry, Stanford University, Stanford, California 94305, United States Yin-Hung Lai Yin-Hung Lai Department of Chemistry, Stanford University, Stanford, California 94305, United States Department of Chemical Engineering, National United University, Miaoli, Taiwan 360, Republic of China Garrett A. Wadsworth Garrett A.

Single liquid-phase and liquid-liquid phase reactions in microdroplets have shown much faster kinetics than that in bulk phase. This work extends the scope of microdroplet reactions to gas-liquid reactions and achieves preparative synthesis. We report highly efficient aerobic oxidation of aldehydes to carboxylic acids in microdroplets. Molecular oxygen plays two roles: (1) as the sheath gas to shear the aldehyde solution into microdroplets, and (2) as the sole oxidant.