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Hydrogel Electrolyte Film with Low‐Temperature Adaptability for Flexible Quasi‐Solid‐State Batteries
Conflict of Interest The authors declare no conflict of interest. Supporting Information Filename Description smll202502243-sup-0001-SuppMat.docx6.5 MB Supporting Information References 1, , , , , Natl. Sci. Rev. 2021, 8, nwaa261. 2, , , , , , , , J. Mater. Chem. A 2024, 12, 21531. 3, , , , , Electrochi. Acta 2019, 320, 134571. 4, , , , , , , , Mater. Futures 2024, 3, 025101. 5, , , , , , , , , Angew. Chem., Int. Ed. 2023, 62, 202311589. 6, , , , Energy Storage Mater. 2024, 72, 103707.
Flexible All‐in‐one Quasi‐Solid‐State Batteries Enabled by Low‐water‐content Hydrogel Films
Abstract The high conductivities and good mechanical properties of hydrogel electrolyte films are critical for energy storage devices with high flexibility, fast redox kinetics, and long life. Herein, a low water content (6.63 wt%) hydrogel film is prepared, and a favorable environment is created, with an electrochemical stability window of 2.26 V and a high ionic conductivity of 2.6 mS cm−1. The hydrogel film exhibits good folding ability, low in-plane swelling, and anti-freezing abilities.
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