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Operando insights on stable Cu 2+ active sites for efficient electrochemical CO 2 -to-C 2 H 4 conversion
Abstract Copper catalysts feature unique superiorities for the electrochemical conversion of CO2 to C2+ fuels and chemicals. Their surface oxidation states dominantly determine the reaction pathways to various products. However, most Cu-based catalysts inevitably undergo electroreduction from Cu2+ to Cu1+ or Cu0 species during the electrochemical CO2 reduction.
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