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Abstract Nuclear magnetic resonance is a powerful tool for applications ranging from chemical analysis to quantum information processing. Achieving optical initialization and detection of molecular nuclear spins promises new opportunities—including improved nuclear magnetic resonance signals at low magnetic field, sensitivity down to the single-molecule level and full access to atomically precise molecular architectures for quantum technologies.
Abstract Optically addressable solid-state spins have been extensively studied for quantum technologies, offering unique advantages for quantum computing, communication, and sensing. Advancing these applications is generally limited by finding materials that simultaneously provide lifetime-limited optical and long spin coherences. Here, we introduce 171Yb3+ ions doped into a CaWO4 crystal.