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Synergy of Ni single atoms and NiO nanoclusters in carbon nitride to create local charge polarization for enhanced CO2 photoreduction
Carbon dioxide photoreduction (CO2PR) enables solar energy conversion into fuels, holding great promise for advancing carbon neutrality [1], [2]. Nonetheless, the efficiency of CO2PR activity is hindered by the challenges of activating nonpolar CO2 molecules and cleaving strong C=O double bonds with a high dissociation energy (∼750 kJ mol−1) [3], [4].
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