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Manipulatable Cascade Pumping Single-Photon Upconversion
Abstract Photon upconversion (UC), while promising for infrared photonics, is fundamentally constrained by limited spectral response range, low efficiency, and slow response speeds. Here, we present a machine learning-guided single-photon UC strategy based on cascade pumping that implements a “LEGO-inspired photon stacking” mechanism, in which intermediate state of lanthanide ions (Ln3+) becomes a “virtual ground state” for direct single-photon pumping to target energy levels.
Dynamic Upconversion Manipulation via Cross‐Relaxation Engineering for Optical Encryption
Conflicts of Interest The authors declare no conflicts of interest. Data Availability Statement All data needed to evaluate the conclusions in the paper are present in the paper and/or the Supplementary Materials. Supporting Information Filename Description adma72400-sup-0001-SuppMat.docx19 MB Supporting File 1: adma72400-sup-0001-SuppMat.docx. adma72400-sup-0002-MovieS1.mov4.3 MB Supporting File 2: adma72400-sup-0002-MovieS1.mov.
Dynamic Multicolor Upconversion Through Excitation Pulse Duration Modulation toward Machine Learning Assisted Optical Encryption
Conflict of Interest The authors declare no conflict of interest. Supporting Information Filename Description lpor202500465-sup-0001-SuppMat.docx2.7 MB Supporting Information References 1, , , , , , , Sci. Adv. 2021, 7, abg0363. 2, , , , , , , , Nat. Commun. 2020, 11, 5484. 3, , , , , , , , , Nat. Commun. 2023, 14, 7298. 4, , , , , , , , Laser Photonics Rev. 2021, 15, 2000343. 5, , , , , Coord. Chem. Rev. 2020, 415, 213328. 6, , , , , , , Light: Sci. Appl. 2021, 10, 140. 7, , , , , , , Adv. Mater. 2023, 36, 2310524.
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