Yu Lan
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Articles by Yu Lan
Study on the effect of nitriding gas on the direct nitridation of silicon swarf from the photovoltaic industry for synthesizing silicon nitride
?Mathematical formulae have been encoded as MathML and are displayed in this HTML version using MathJax in order to improve their display. Uncheck the box to turn MathJax off. This feature requires Javascript. Click on a formula to zoom. ABSTRACT In the process of diamond wire cutting silicon wafers in the photovoltaic industry, tens of thousands of tons of high-purity silicon swarf are generated. There is an urgent need for the recycling and utilization of silicon swarf.
A unified and desymmetric approach to axially chiral atropisomers
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Abstract Given the widespread applications of axially chiral atropisomers, the development of catalytic asymmetric transformations toward their preparation has been an important goal in organic synthesis and is under intensive investigation.
By Dan Hu, Yu Huang, Wenxuan Lin, Tao Zhang, Penghui Li, Zihao Jiao, Linghui Qian, Yu Lan, Xin Li Verified, Jia-Yu Liao
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Nature
Verified
RACK1 maintains mouse hematopoietic stem cells by directly binding to and stabilizing LDB1
Abstract A core complex with transcription factors (TFs) TAL1/TCF3/GATA2 and adaptors LMO2/LDB1 lies at the top of the hematopoietic transcriptional hierarchy. The mechanism(s) underlying the expression of these components remain elusive. Adaptor RACK1 interacts with multiple TFs and modulates their activation and/or stability. However, a role of RACK1 in the transcriptional control of hematopoietic stem cell (HSC) fates hasn’t been disclosed.
Synthesis and Properties of Silicone-Modified Iodonium Salt Photoinitiators Click to copy article link Article link copied!
Abstract Click to copy section linkSection link copied! Silicone materials exhibit excellent weatherability, heat resistance, biocompatibility, and low surface tension, showing broad application prospects. Photocuring technology, known for its high efficiency, energy savings, and environmental friendliness, has become a key approach for preparing silicone polymers.
Mechanism-Inspired Chiral Binuclear Cu Catalysis for Click Chemistry: Highly Efficient Kinetic Resolution to α-Quaternary Amino Acid Derivatives Click to copy article link Article link copied!
Cite Jump to ExpandCollapse ArticleJune 29, 2026 Mechanism-Inspired Chiral Binuclear Cu Catalysis for Click Chemistry: Highly Efficient Kinetic Resolution to α-Quaternary Amino Acid Derivatives Click to copy article linkArticle link copied! Zekai Fang Zekai Fang State Key Laboratory of Organometallic Chemistry and Shanghai-Hongkong Joint Laboratory in Chemical Synthesis, Shanghai Institute of Organic Chemistry, University of Chinese Academy of Sciences, Chinese Academy of Sciences, 345...
Epiblast diversification and blood formation in a human pregastrula
Abstract The incipient stage of gastrulation in human, when the primitive streak is about to emerge, represents a critical yet underexplored period. Here we present the high-resolution spatial transcriptomic landscape of a human embryo at Carnegie stage 6 (approximately 13–14 days post-conception), a stage at which primitive streak remains invisible and gastrulation-derived mesodermal/endodermal progenitors are not yet transcriptomically detected.
Targeting MEF2A suppresses microglial hyperactivation and synaptic phagocytosis to attenuate epilepsy pathogenesis
Abstract Microglia’s role in epilepsy through neuroimmune communication is poorly understood. Mechanisms by which neurons activate microglia and how microglia affect neuronal activity to drive seizure-related inflammation remain unclear. Here, we elucidated a crucial axis connecting pathological adenosine triphosphate (ATP) release induced by epileptiform neuronal activity to microglial MEF2A-dependent hyperactivation, which exacerbates epilepsy pathology.
Theoretical Study and Rational Design of Noncovalent Interactions Enable Organocatalytic Divergent [2+2] and [4+2] Annulations Click to copy article link Article link copied!
Cite Jump to ExpandCollapse LetterMay 7, 2026 Theoretical Study and Rational Design of Noncovalent Interactions Enable Organocatalytic Divergent [2+2] and [4+2] Annulations Click to copy article linkArticle link copied! Xinghua Wang Xinghua Wang Henan Engineering Laboratory of Green Synthesis for Pharmaceuticals, College of Chemistry and Chemical Engineering, Shangqiu Normal University, Shangqiu, Henan 476000, P. R.
Individualized duration of adjuvant alectinib therapy and rechallenge efficacy in ALK-positive non-small cell lung cancer: a case report
Abstract Background: Anaplastic lymphoma kinase (ALK)-rearranged non-small cell lung cancer (NSCLC) is a distinct molecular subtype of cancer that typically affects younger patients and carries a high risk of central nervous system (CNS) metastases. Adjuvant alectinib therapy has demonstrated efficacy in prolonging disease-free survival; however, the optimal duration of adjuvant treatment remains undefined.
Antioxidant, Degradable, and 3D-Printable Hydrogels Enabled by a Gelatin-Flavin Conjugate Photoinitiator Click to copy article link Article link copied!
Abstract Click to copy section linkSection link copied! The development of novel photoinitiators possessing both photopolymerization activity and biological functionality has become a critical challenge in advancing hydrogel applications in biomanufacturing and precision medicine. Particularly in the fabrication of high-resolution 3D-printed hydrogel constructs, the properties of photoinitiators directly determine polymerization efficiency, printing success, and structural resolution.
Quantifying the spatiotemporal dynamics of the first two epidemic waves of SARS-CoV-2 infections in the United States
Citation: Lopes R, Lan Y, Chitwood MH, Klaassen F, Salomon JA, Menzies NA, et al. (2026) Quantifying the spatiotemporal dynamics of the first two epidemic waves of SARS-CoV-2 infections in the United States. PLoS Comput Biol 22(3): e1013983. https://doi.org/10.1371/journal.pcbi.1013983 Editor: Claudio José Struchiner, Fundação Getúlio Vargas: Fundacao Getulio Vargas, BRAZIL Received: January 14, 2025; Accepted: February 4, 2026; Published: March 4, 2026 Copyright: © 2026 Lopes et al.
Asymmetric synthesis of enantioenriched lactams from cyclic ketones via Beckmann rearrangement - Nature Chemistry
Abstract The direct incorporation of a single nitrogen atom into ketones or aldehydes represents one of the most valuable transformations for constructing amides and lactams, motifs that are ubiquitous in pharmaceutical manufacturing and industrial synthesis. Despite its importance, achieving precise stereochemical control in this process remains a formidable and long-standing challenge, primarily owing to the demanding reaction conditions typically required for such transformations.
Photoinduced polarity-mismatched transformations of isoquinolines into naphthalenes - Nature Communications
Abstract Isosteric replacement is an important strategy for lead optimization in drug-development paradigms. However, it is usually restricted to cost- and labor-intensive de novo syntheses. We here report a photochemical photosensitizer-free skeletal-editing strategy to directly transform easily accessible isoquinolines into synthetically challenging naphthalene derivatives in a single operation.
Evolution of manganese low-energy photoredox catalysis from high-energy visible light photocatalysis - Nature Communications
Abstract Reducing the energy input of light in photocatalytic reactions is desirable yet challenging, as modifying the light-absorbing or catalytic properties of a photocatalyst typically requires tedious preparation, resulting in a lengthy development process. Here, we overcome this limitation by achieving manganese-based low-energy photoredox catalysis through the in-situ assembly of simple Mn salts with inexpensive coordinating chemicals, thereby bypassing the need for complex pre-preparation.
The Origin of Stereoselectivity in Dual Transition‐Metal/NHC Asymmetric Catalysis: A Competitive Induction Model
Supporting Information Filename Description cjoc202501259-sup-0001-supinfo.pdfPDF document, 2.1 MB Appendix S1: Supporting Information References 1 Asymmetric catalysis: An enabling science. Proc. Natl. Acad. Sci. 2004, 101, 5348–5355. 2 ; ; ; ; ; ; ; ; ; Recent Progress of Asymmetric Catalysis from a Chinese Perspective. CCS Chem. 2023, 5, 2685–2716. 3 ; Stereodivergence in Asymmetric Catalysis. J. Am. Chem. Soc. 2017, 139, 5627–5639. 4 ; ; ; ; Theory and Modeling of Asymmetric Catalytic Reactions. Acc. Chem.
β-Sulfinimidoyl Esters as Sulfenamide Anion Precursors for Accessing Aza-Sulfur Stereogenic Centers
Organic Letters Cite this: Org. Lett. 2025, XXXX, XXX Click to copy citationCitation copied! Learn about these metrics Article Views are the COUNTER-compliant sum of full text article downloads since November 2008 (both PDF and HTML) across all institutions and individuals. These metrics are regularly updated to reflect usage leading up to the last few days. Citations are the number of other articles citing this article, calculated by Crossref and updated daily.
Copper-catalysed homo-Mannich reaction of cyclopropanol for chiral piperidine synthesis - Nature Catalysis
Abstract The Mannich reaction represents one of the most fundamental reactions for the stereoselective synthesis of β-amino-carbonyl compounds and has been broadly applied in organic synthesis. In contrast, the homologue of the Mannich reaction, the so-called the homo-Mannich reaction, which generates the homologated γ-amino-carbonyl products, remains largely underexplored despite its potential for diverse applications.
Divergent access to E- or Z-trisubstituted medium-sized cycloalkenes by Pd-catalysed cycloaddition - Nature Chemistry
Abstract Despite their significance in nature, medium-sized rings (particularly 9–11 membered ones) are non-existent in commercial small-molecule drugs largely due to the lack of efficient syntheses. Even with the widespread presence of macrocyclic alkenes in therapeutic agents, stereoselective access to either E- or Z-alkenes remains a formidable challenge.
Thiophenol-Catalyzed Radical Hydroformylation of Unactivated Sterically Hindered Alkenes
Cite Jump to ExpandCollapse ArticleAugust 21, 2025 Thiophenol-Catalyzed Radical Hydroformylation of Unactivated Sterically Hindered Alkenes Click to copy article linkArticle link copied! Yisicheng Wang Yisicheng Wang State Key Laboratory of Chemical Biology, Shanghai Institute of Organic Chemistry, University of Chinese Academy of Sciences, 345 Lingling Road, Shanghai 200032, China School of Physical Science and Technology, ShanghaiTech University, 100 Haike Road, Shanghai 201210, China...
Advancing PbS Quantum Dot Superlattice for High-Performance Electrical Transport and Infrared Photodetection Integrated with Two-Dimensional MoS₂ The optoelectronics field has recently experienced a notable surge in research focused on hybrid structures that integrate colloidal quantum dots (QDs) with two-dimensional (2D) materials.
Discord between ‘Maghrebi brothers’: Morocco-Algeria interstate and intrastate conflicts, 1962-1964
ABSTRACT This article assesses the origins, causes, and consequences of the deteriorating Morocco-Algeria relations in the early 1960s. It begins by examining the role of colonial legacy and decolonisation processes, which laid the foundation for two ideologically contrasted regimes in the Maghreb – the Alaouite monarchy in Morocco and a leftist republic in Algeria.
Human yolk sac-derived innate lymphoid-biased multipotent progenitors emerge prior to hematopoietic stem cell formation
Main text (Developmental Cell 59, 2626–2642.e1–e6; October 7, 2024) In our recent paper entitled “Human yolk sac-derived innate lymphoid-biased multipotent progenitors emerge prior to hematopoietic stem cell formation” (DEVCEL_5945), we regret that in supplementary figure 5, the last two panels of the representative flow cytometry plots for CD127– clonal output (ILC-Mono/Mac-Mast cell-cDC (18)) were inadvertently duplicated in the CD127+ clonal output (ILC-Mono/Mac-cDC (4)) section, as well...
Renewable Photosensitive Castor Oil to Fabricate Ionogels: Freezing‐Tolerance, Stretchability, and Degradation for 3D Printing and Flexible Sensor Applications
Conflict of Interest The authors declare no conflict of interest. Supporting Information Filename Description smll202502700-sup-0001-SuppMat.docx2.6 MB Supporting Information References 1, , Nat. Rev. Mater. 2018, 3, 125. 2, , , Mater. Horiz. 2020, 7, 912. 3, , , , , , , , Chem. Eng. J. 2024, 483, 149330. 4, , , , , , , Science. 2020, 370, 961. 5, , , , , , , , , , Nature. 2021, 590, 594. 6, , , , , , , , Macromolecules. 2022, 55, 10950. 7, , , , , , , , , , J. Am. Chem., Soc. 2024, 146, 13903.
How to Achieve Hydrogenation/Hydrofunctionalization via Metal Hydride Complexes
Abstract Click to copy section linkSection link copied! Conspectus Metal hydride (M–H) complexes have garnered widespread attention in the synthesis of fine chemicals, materials, agrochemicals, and pharmaceuticals owing to the remarkable reactivity of the M–H bonds.
How to Achieve Hydrogenation/Hydrofunctionalization via Metal Hydride Complexes
Abstract Click to copy section linkSection link copied! Conspectus Metal hydride (M–H) complexes have garnered widespread attention in the synthesis of fine chemicals, materials, agrochemicals, and pharmaceuticals owing to the remarkable reactivity of the M–H bonds.
新加坡新激励措施助力资本市场长期增长
新加坡证券市场研究小组[2]在2025年2月21日发布了首个提振新加坡资本市场的系列措施[3]，包括推出50亿新币的证券市场发展计划（Equity Market Development Programme，“EQDP”）、加快和简化企业上市流程等。发布的措施中还重申了此前黄循财总理在2025年财政预算案中提到的有关税收激励[4]。 领导证券市场研究小组的新加坡交通部长兼财政部第二部长、金融管理局副主席徐芳达在当天的记者会上表示[5]，目前全球资本及流动性仍主要集中在少数全球性交易所（尤其是美国的交易所）中，这些市场也吸引了大量投资者和公司的目光；相比之下，新加坡等的本地股市在吸引上市、增强流动性方面面临着重大的挑战，导致近年来新优质公司上市数量偏少、交易量偏低[6]。证券市场研究小组希望通过着眼于强化本地证券市场生态环境的建设以及提升证券市场吸引力，使企业将新加坡视作获得融资、实现长期稳定成长的理想目的地；同时希望借助新加坡活跃的初创企业、成熟的PE/VC和基金管理生态系统，将新加坡资本市场打造成为适合中小型企业融资与成长的理想市场。...
新加坡2025财政预算：强化企业投资与科技创新，助力未来经济可持续增长
2025年2月18日，新加坡总理黄循财在国会发表了2025年财政预算声明，主题为“齐心前进，迈向未来”[2]。此次预算案旨在应对全球经济挑战，提升国家竞争力；在新加坡建国60周年之际，为新加坡公民提供多项福利，也在多方面采取增强新加坡投资吸引力、科技竞争力及改善营商环境的举措。本文主要梳理了财政预算有关营商环境、投资促进、科技创新等方面的利好政策和措施，为投资者前往新加坡开展投资活动提供参考。 一、应对全球经济挑战，新加坡表现依旧亮眼 黄总理介绍，新加坡去年经济表现强劲，GDP增长达到4.4%，通货膨胀持续放缓。居民就业人口的收入中位数增长比通胀率高出3.4%。新加坡2024年基尼系数为0.364[3]，贫富差距降至2000年以来最低水平[4]。但鉴于全球不确定性和经济下行的风险日渐增加，新加坡2025年的经济增速预期将放缓至1%至3%，平均通胀率预计为1.5%至2.5%。 二、企业优惠：公司税收回扣与加薪补贴...
Desymmetrization of 1,4‐Diynes by Allylic Alcohol‐Triggered Redox Enyne Cycloisomerization
Supporting Information As a service to our authors and readers, this journal provides supporting information supplied by the authors. Such materials are peer reviewed and may be re-organized for online delivery, but are not copy-edited or typeset. Technical support issues arising from supporting information (other than missing files) should be addressed to the authors.
Organocatalytic enantioselective synthesis of double S-shaped quadruple helicene-like molecules - Nature Communications
Abstract Helicene-shaped molecules are compelling chemical structures with unique twisted helical chirality and remarkable properties. Although progress occurs in the catalytic asymmetric synthesis of helicene (-like) molecules, the enantioselective synthesis of multiple helicenes, especially four or higher helicity, is still challenging and has yet to be achieved.
An agile multimodal microrobot with architected passively morphing wheels
Research Article APPLIED SCIENCES AND ENGINEERING INTRODUCTION Microrobots (1) (length < 15 cm, mass < 20 g) with the ability to perform multimodal locomotion (1–9) can navigate across various unstructured environments and accommodate terrain changes, holding promising potential for a broad spectrum of applications, such as inspection (5, 10), exploration (1, 6), rescue tasks (11, 12), and biomedicine (5, 13–17).
Backbone Engineering of Indacenodithiophene-Based Polymers for High-Performance Vertical Organic Electrochemical Transistors and Efficient Glucose Sensor
Abstract Click to copy section linkSection link copied! Organic mixed ionic-electronic conductors (OMIECs) play a fundamental role in the performance of organic electrochemical transistors (OECTs) and their applications. Although several depletion mode and accumulation mode OMIECs have been utilized for efficient OECT-based glucose sensors, there are still persistent drawbacks such as including biocompatibility, instability, or high detection limits.
Dual Ligands Unlocking Iron and Halogen-Containing Carboxylates-based Photocatalysis for Chloro/Fluoro-Polyhaloalkylation of Alkenes
Dual Ligands Unlocking Iron and Halogen-Containing Carboxylates-based Photocatalysis for Chloro/Fluoro-Polyhaloalkylation of Alkenes Herein, we demonstrate a practical dual ligand-enabled iron photocatalysis paradigm—translating all kinds of halogen-containing carboxylates (CnXmCOO−, X: F, Cl, Br) into CnXm radicals for the valuable chloro/fluoro-polyhaloalkylation of non-activated alkenes with easily available trichloroacetonitrile/Selectfluor as the electrophilic halogenation reagent.
Will NATO annual nuclear exercise "Steadfast Noon" once again shroud Europe in the shadow of nuclear war?
By Yu Lan NATO kicked off its large-scale nuclear exercise "Steadfast Noon" in northern Europe on Monday, with 2,000 soldiers and 60 aircraft from 13 NATO countries participating in the exercise. NATO Secretary General Mark Rutte said, "Steadfast Noon sends a clear message to any adversary that NATO will protect and defend all Allies." This year's exercise, hosted by Belgium and the Netherlands, involves participants simulating missions in which fighter jets carry US nuclear warheads.
"Semiparametric Copula-Based Regression Modeling of Semi-competing Risk" by Hong Zhu, Yu Lan et al.
Abstract Semi-competing risks data often arise in medical studies where the terminal event (e.g., death) censors the non-terminal event (e.g., cancer recurrence), but the non-terminal event does not prevent the subsequent occurrence of the terminal event. This article considers regression modeling of semi-competing risks data to assess the covariate effects on the respective non-terminal and terminal event times.
Theoretical study on ligand conformational self-adaptation for modulating reactivity - Scientific Reports
Abstract The combination of Josiphos-type ligands with Pd catalysts has been instrumental in the rapid development of efficient catalytic processes. We performed density functional theory (DFT) calculations to elucidate the mechanisms and dynamic conformational changes responsible for the reactivity and selectivity observed in Pd-catalysed bicyclization/carbonylation of 1,6-enynes.
Bifunctional iron-catalyzed alkyne Z-selective hydroalkylation and tandem Z-E inversion via radical molding and flipping - Nature Communications
Abstract The challenging synthesis of thermodynamic-unfavored cis-olefins through catalytic cross-coupling reactions requires the synergistic interaction of substrate-activating units and configuration-regulating catalysts. Successfully hitting these two birds with one stone, we herein develop a convenient photoredox access to Z-alkenes from alkynes and light alkanes with a bifunctional iron-catalyzed system possessing both C(sp3)−H activation and configuration-controlling abilities.
Long‐Term Biochar Application Improved Aggregate K Availability by Affecting Soil Organic Carbon Content and Composition
Conflicts of Interest The authors declare no conflicts of interest. References , , , et al. 2023. “Increased Humic Materials Explain Aggregate-Protected Carbon and Nitrogen Accumulation in Biochar-Amended Tropical Soils.” Pedosphere. https://doi.org/10.1016/j.pedsph.2023.07.006. , , and . 2002. “Enhancement of Copper and Cadmium Adsorption on Kaolin by the Presence of Humic Acids.” Chemosphere 48: 1081–1088. https://doi.org/10.1016/S0045-6535(02)00169-8. , , , et al. 2024.
Differentiation Across Bipolar Disorder and Major Depressive Disorder by Whole-Night Polysomnographic Findings
Abstract Background: There is growing evidence that understanding the role of sleep disturbance in bipolar disorder (BD) and major depressive disorder (MDD) is helpful when studying the high heterogeneity of patients across psychiatric disorders. Objective: The present study was designed to investigate the transdiagnostic role of sleep disturbance measured by polysomnography (PSG) in differentiating from MDD with BD.
Synthesis and Biological Activities of C1-Substituted Acylhydrazone β-Carboline Analogues as Antifungal Candidates
1. Introduction Plant pathogenic fungi have long been considered one of the main causative agents of plant diseases. They can infect any tissue at different stages of plant growth, leading to serious declines in the quality and yield of agricultural products. Several fungi-caused plant diseases have become major problems worldwide, including those caused by Valsa mali, Fusarium graminearum, Fusarium oxysporum, and Fusarium solani [1].
Enantioselective de novo construction of 3‑oxindoles via organocatalyzed formal [3 + 2] annulation from simple arylamines - Nature Communications
Abstract The de novo construction of enantioenriched 3-hydroxyindolenines and 3-oxindoles from easily available starting materials has been highly desired. Herein, an enantioselectively intermolecular direct [3 + 2] annulation of aryl amine with 2,3-diketoesters to construct 3-hydroxyindolenines with a chiral tertiary alcohol has been disclosed.
Iron photocatalysis via Brønsted acid-unlocked ligand-to-metal charge transfer - Nature Communications
Abstract Reforming sustainable 3d-metal-based visible light catalytic platforms for inert bulk chemical activation is highly desirable. Herein, we demonstrate the use of a Brønsted acid to unlock robust and practical iron ligand-to-metal charge transfer (LMCT) photocatalysis for the activation of multifarious inert haloalkylcarboxylates (CnXmCOO−, X = F or Cl) to produce CnXm radicals.
US, Russia's medium-range missile gaming triggers arms race
By Yu Lan America's deployment of medium and short-range missiles in the Asia Pacific and Europe has put Russia and other countries on high alert. Moscow has repeatedly warned that if the US deployed land-based medium and short-range missiles in the Asia Pacific and Europe, it would maintain the right to unilaterally suspend the Intermediate-Range Nuclear Forces (INF) Treaty.
Chemo-, regio- and stereoselective access to polysubstituted 1,3-dienes via Nickel-catalyzed four-component reactions - Nature Communications
Abstract 1,2-Difunctionalization of alkynes offers a straightforward approach to access polysubstituted alkenes. However, simultaneous multi-component cascade transformations including difunctionalization of two alkynes with both syn- and anti-selectivity in one catalyst system is undeveloped and proves to be a significant challenge.
Development of a New Positron Emission Tomography Imaging Radioligand Targeting RIPK1 in the Brain and Characterization in Alzheimer's Disease
1 Introduction Apoptosis is a form of caspase-dependent non-inflammatory programmed cell death that is strictly regulated by intracellular signaling molecules[1] Unlike apoptosis, necrosis is a type of non-programmed cell death that is a passive death mode that occurs under uncontrollable extreme external conditions.[2, 3] These two forms of cell death have been regarded as the primary forms of cell death in recent decades.
Asymmetric hydrogenation of ketimines with minimally different alkyl groups - Nature
Abstract Asymmetric catalysis allows the synthesis of optically active compounds, often requiring the differentiation between two substituents on prochiral substrates1. Despite decades of development of mainly noble metal catalysts, achieving differentiation between substituents with similar steric and electronic properties remains a significant challenge2,3.
Effects of Selenium Incorporation on the Performance of Polythiophene Based Organic Electrochemical Transistors
Effects of Selenium Incorporation on the Performance of Polythiophene Based Organic Electrochemical Transistors Selenium incorporation is a widely used strategy for achieving high mobility semiconductors for a variety of organic optoelectronic devices, but it has received less attention in organic electrochemical transistors (OECTs).
Umpolung reactivity of strained C–C σ-bonds without transition-metal catalysis - Nature Communications
Abstract Umpolung is an old and important concept in organic chemistry, which significantly expands the chemical space and provides unique structures. While, previous research focused on carbonyls or imine derivatives, the umpolung reactivity of polarized C–C σ-bonds still needs to explore.
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