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Articles by Shaobin Wang
UPMA: unspecified pretraining and modular adaptation for context-aware target delineation in adaptive esophageal radiotherapy
Abstract Esophageal cancer, a serious malignancy, is primarily treated with radiotherapy (RT). Accurate delineation of gross tumor volume (GTV) and clinical target volume (CTV) is essential, yet manual contouring is time-consuming and automatic methods remain challenging. Adaptive radiotherapy enables personalized target adjustments, but tumor changes following initial RT complicate delineation, and automatic second-phase replanning is underexplored.
Decoding Synergistic Pathways in Bimetallic MOFs for Advanced Oxidation Processes
2.1.2.1 Hard–Soft Acid–Base (HSAB) Principle Bond strength can be described and governed by the HSAB principle, which states that hard acids preferentially bind hard bases, and soft acids bind soft bases [77-80]. In MOF chemistry, carboxylate-binding ligands (hard bases) form strong bonds with high-valent metal ions (hard acids), such as Cr(III), Al(III), Fe(III), Ti(IV), Zr(IV), and Mn(IV).
Engineering N-site isomerism in donor-acceptor covalent organic frameworks for efficient Fenton-like water purification
Abstract Covalent organic frameworks (COFs) have emerged as promising candidates for singlet oxygen (1O2) generation via peroxymonosulfate (PMS) activation, yet their structure-property-activity relationships remain poorly understood. Herein, three constitutionally isomeric donor-acceptor COFs (TF-22Bpy, TA-22Bpy and TA-33Bpy) were constructed via N-site isomeric engineering, which involved precisely modulation of the imine and pyridine nitrogen positions within the skeleton.
Materials Design for Environmental Technologies: Advancing Water and Air Purification Through Functional Materials Innovation
Opens in a new window Opens an external website Opens an external website in a new window This website utilizes technologies such as cookies to enable essential site functionality, as well as for analytics, personalization, and targeted advertising. To learn more, view the following link: Privacy Policy Advanced Hub Main Navigation Menu Weng, B., Wang, S., Zheng, Y.-M., Choi, W. and Caro, J.
Dynamic variations of metal-O bonding in electro- and thermo-catalytic activation processes
Abstract Dynamically tracking the variations in electronic configurations and molecular binding of a catalyst under operando conditions remains a significant challenge. Herein, we report an in-situ millisecond-resolved wide-angle X-ray scattering technique to capture lattice distortion within a catalyst in low-temperature oxidation under electric- and thermal-induced catalysis and reveal the intrinsic mechanism of metal-O bonding on oxygen activation and the electro promotion.
Axial oxygen coordination drives spin-regulated electron transfer in single-atom Fe catalysts for selective pollutant transformation
Abstract Precise modulation of spin states of single-atom catalysts (SACs) offers a promising route to fine-tune peroxide activation behaviors and selectivity toward different oxidation pathways. Here, we report a spin-tunable Fe SAC composed of iron phthalocyanine (FePc) axially coordinated via oxygen bridges (-O-) onto annealed nanodiamond (AND), denoted as FePc-O-AND. The axial oxygen coordination induces a spin transition from high-spin (t2g5eg3) to an intermediate-spin (t2g4eg2) state.
An asymmetric photothermal platform for coupled seawater splitting and desalination
Abstract Photocatalytic seawater splitting provides a sustainable route to green hydrogen, but faces barriers of inefficiency and scalability. Graphitic carbon nitride (g-C3N4, CN) offers saline tolerance, yet its catalytic potential requires atomic-level control of structure and charge dynamics. Herein, we design three single-atom Co configurations on CN, including symmetric Co–N4, vacancy-anchored Co–N3, and asymmetric Co–N4.
Integrating Economic Vitality and Cultural Identity Heritage Revitalization of Lingnan Commercial Qilou Architecture across the Guangdong-Hong Kong-Macao Region
1. Introduction The arcade, or Qilou (骑楼), is one of the most distinctive architectural forms in the Lingnan region of South China. Developed during the late Qing dynasty and flourishing throughout the Republican period, this typology combines commercial functionality with cultural adaptation. Characterized by continuous covered walkways, open arcades, and hybrid façades (Wu et al., 2025), Lingnan’s arcades reflect a unique fusion of Western colonial influence and traditional Chinese spatial logic.
Best practices for advanced oxidation processes - Nature Sustainability
Lack of transparency and standardization in experimental design and performance evaluation hinders the real-world applications of advanced oxidation processes — critical technologies in wastewater treatment. Here, we highlight the common pitfalls in advanced oxidation process research and propose practices to guide future studies.
Photo-assisted technologies for environmental remediation - Nature Reviews Clean Technology
Abstract Industrial processes can lead to air and water pollution, particularly from organic contaminants such as toluene and antibiotics, posing threats to human health. Photo-assisted chemical oxidation technologies leverage light energy to mineralize these contaminants. In this Review, we discuss the mechanisms and efficiencies of photo-assisted advanced oxidation processes for wastewater treatment and photothermal technologies for air purification.
Correction: Atomically dispersed cobalt on graphitic carbon nitride as a robust catalyst for selective oxidation of ethylbenzene by peroxymonosulfate
Correction: Atomically dispersed cobalt on graphitic carbon nitride as a robust catalyst for selective oxidation of ethylbenzene by peroxymonosulfate Correction for ‘Atomically dispersed cobalt on graphitic carbon nitride as a robust catalyst for selective oxidation of ethylbenzene by peroxymonosulfate’ by Jiaquan Li et al., J. Mater. Chem. A, 2021, 9, 3029–3035, https://doi.org/10.1039/D0TA11503G. This article is Open Access This article has not yet been cited.
The Aesthetic Imagery of Traditional Garden Door and Window Forms: A Case Study of the Four Major Traditional Gardens of Lingnan
1. Introduction 1.1. Background Traditional Lingnan gardens are one of the three major types of classical Chinese gardens, along with northern and southern gardens. Lingnan gardens are affected by their geographical environment and the considerable influences of culture and economy, resulting in unique regional style characteristics. The types and styles of the doors and windows, important parts of the building facades in Lingnan gardens, profoundly affect the overall atmosphere of the gardens.
Synergistic effects of metallic IrCo for promoted nitrate reduction in industrial-relevant wastewater level
Nitrate ions, as one of most widespread pollutants in wastewater streams, pose significant hazards to human health and aquatic ecosystem biodiversity [1], [2]. They are commonly derived from agricultural activities, industrial discharges and urban sewage systems, while the concentration of nitrate ranges from hundreds to thousands ppm [3], [4], [5]. Crucially, removal of nitrate in wastewater is a pressing task to maintain global nitrogen cycle.
Mechanistic insights into ultrafast degradation of electron-rich emerging pollutants by waste cyanobacteria resource utilization
At present, there are many antibiotics and other difficult to degrade organic pollutants in the wastewater of agriculture and livestock, which will be harmful to the water environment and human body with the water circulation if they flow into the lake for a long time [1], [2]. Advanced oxidation process (AOP) is highly effective in treating hard-to-degrade pollutants in water, including electrocatalytic, photocatalytic, Fenton-like, and so on [3], [4].
Contemporary Demands of Scenes in Urban Historic Conservation Areas: A Case Study of Subjective Evaluations from Foshan, China
1. Introduction The focus of this research is to examine how historical areas adapt to the demands of modern society during the process of urban development, and identify potential points for optimization to achieve a harmonious balance between preservation and progress.
Size‐Dependent Catalysis in Fenton‐like Chemistry: From Nanoparticles to Single Atoms
State-of-the-art Fenton-like reactions are crucial in advanced oxidation processes (AOPs) for water purification. This review explores the latest advancements in heterogeneous metal-based catalysts within AOPs, covering nanoparticles (NPs), single-atom catalysts (SACs), and ultra-small atom clusters.
Highly efficient micropollutant decomposition by ultrathin amorphous cobalt-iron oxide nanosheets in peroxymonosulfate-mediated membrane-confined catalysis
Water pollution, primarily caused by human activities, has significant economic and health implications [1], [2]. It disrupts the smooth functioning of sectors such as agriculture and industries. It is included in the United Nations' sustainable development goals, specifically those related to clean water (SDG6) and good health (SDG3).
Dual Nonradical Catalytic Pathways Mediated by Nanodiamond-Derived sp2/sp3 Hybrids for Sustainable Peracetic Acid Activation and Water Decontamination
Download Hi-Res ImageDownload to MS-PowerPointCite This:Environ. Sci. Technol. 2024, XXXX, XXX Terms & Conditions Most electronic Supporting Information files are available without a subscription to ACS Web Editions. Such files may be downloaded by article for research use (if there is a public use license linked to the relevant article, that license may permit other uses).
Study on the Influence Factors of the Dynamic Property of the Polyurethane Mixture with Dense Gradation
4.1. Comparing Master Curve Fitting Results 4.1.1. The GLS Model Fitting Results for Dynamic Modulus Figure 2a,b demonstrate that the PU mixtures with various limestone gradations exhibited distinct dynamic modulus master curves. The master curve of PUM-20/L was lower than the other master curves.
Rapid self-heating synthesis of Fe-based nanomaterial catalyst for advanced oxidation - Nature Communications
Abstract Iron-based catalysts are promising candidates for advanced oxidation process-based wastewater remediation. However, the preparation of these materials often involves complex and energy intensive syntheses. Further, due to the inherent limitations of the preparation conditions, it is challenging to realise the full potential of the catalyst. Herein, we develop an iron-based nanomaterial catalyst via soft carbon assisted flash joule heating (FJH).
Perspectives of Wood-Inspired Electro-Fenton Catalysis for Energy-Efficient Wastewater Decontamination
A large-scale deployment of electro-Fenton (EF) technology faces significant challenges, including the high cost of catalysts, complex electrode preparation, and limited energy utilization efficiency.
Minireview of Coupled Electrochemical Hydrogen Production and Organic-Oxidation for Low Energy Consumption
Hydrogen production from electrochemical water splitting has attracted great attention due to its supply to green energy. However, commercial alkaline water electrolysis is energy intensive due to inert and large overpotentials of anodic oxygen evolution reaction (OER). Electro-oxidation of organics is an attractive alternative to the OER.
The influence path of community green exposure index on activity behavior under multi-dimensional spatial perception
1. Introduction Human beings, going through evolution over millions of years, have formed a psychological mechanism for adapting to the natural environment.
Study on Mechanism and Verification of Columnar Penetration Grouting of Time-Varying Newtonian Fluids
Abstract : Penetration grouting technology is an important technical means to improve the mechanical properties of gravel soil layers, and the time-varying characteristics of Newtonian fluid viscosity have an important influence on the morphology and effect of penetration grouting. However, these time-varying properties are not considered in the current research on the mechanism of Newtonian fluid penetration grouting.
Enhanced Photodegradation of Rhodamine B Using Visible-Light Sensitive N-TiO2/rGO Composite
Open AccessArticle by Maisari Utami 1,*, Shaobin Wang 2, Febi Indah Fajarwati 1, Siva Nur Salsabilla 1, Tania Amara Dewi 1 and Melinda Fitri 1 1 Department of Chemistry, Faculty of Mathematics and Natural Sciences, Universitas Islam Indonesia, Yogyakarta 55584, Indonesia 2 School of Chemical Engineering and Advanced Materials, University of Adelaide, Adelaide, SA 5005, Australia * Author to whom correspondence should be addressed.
Carbocatalytic ozonation toward advanced water purification
Carbocatalytic ozonation toward advanced water purification Carbon-based catalytic ozonation is state-of-the-art technology with high oxidation capabilities for wastewater remediation, taking advantage of the synergies of direct ozone oxidation and the generated reactive oxygen species (ROS).
Single-atom catalysis in advanced oxidation processes for environmental remediation
Single-atom catalysis in advanced oxidation processes for environmental remediation Yanan Shang,a Xing Xu, *a Baoyu Gao, a Shaobin Wang b and Xiaoguang Duan *b Author affiliations * Corresponding authors a Shandong Key Laboratory of Water Pollution Control and Resource Reuse, School of Environmental Science and Engineering, Shandong University, Jinan 250100, P. R.
Engineered Graphitic Carbon Nitride-Based Photocatalysts for Visible-Light-Driven Water Splitting: A Review
Graphitic carbon nitride (g-C3N4), a polymeric semiconductor, has become a rising star for photocatalytic energy conversion because of its facile accessibility, metal-free nature, low cost, and environmentally benign properties. This work reviews the latest progress of g-C3N4-based materials in visible-light-driven water splitting to hydrogen.
Bidirectional Progressive Optimization of Carbon and Nitrogen Defects in Solar-Driven Regenerable Adsorbent to Remove UV-Filters from Water
Introduction The boom in nanotechnology and amazing breakthroughs in research on functional nanomaterials have provided great promises for their wide application in electronics, photonics, energy generation/storage, and environmental remediation.(1−4) In the design of various materials, defect engineering technology has been recognized as one of the most promising strategies for performance optimization.(5) Defects are inevitably present in materials where the periodic arrangement of atoms or...
Atomically dispersed cobalt on graphitic carbon nitride as robust catalyst for selective oxidation of ethylbenzene by peroxymonosulfate
Atomically dispersed cobalt on graphitic carbon nitride as robust catalyst for selective oxidation of ethylbenzene by peroxymonosulfate You have access to this article Please wait while we load your content... Something went wrong. Try again?
Novel two-dimensional crystalline carbon nitrides beyond g-C3N4: Structure and applications
Novel two-dimensional crystalline carbon nitrides beyond g-C3N4: Structure and applications Tan Li, Chunyang Nie, Zhimin Ao, Hongqi Sun, Taicheng An and Shaobin Wang Abstract Two-dimensional (2D) crystalline carbon nitrides (CxNy) with graphene-like atomic structures but semiconducting nature are new appealing materials, and increasing interest has been garnered on their synthesis, properties, and applications.
Nanostructured manganese oxides: Natural/artificial formation and their induced catalysis for wastewater remediation
Nanostructured manganese oxides: Natural/artificial formation and their induced catalysis for wastewater remediation Manganese oxides, with low toxicity and wide adaptability, have demonstrated as promising catalysts for substituting noble metals/oxides in a diversity of chemical reactions. In environmental remediation, manganese oxides can catalyze peroxides to produce reactive oxygen species (ROS) in an aqueous phase for in situ chemical oxidation (ISCO) and advanced oxidation processes (AOPs).
Recent progress in g-C3N4 quantum dots: synthesis, properties and applications in photocatalytic degradation of organic pollutants
Recent progress in g-C3N4 quantum dots: synthesis, properties and applications in photocatalytic degradation of organic pollutants Teng Wang,†a Chunyang Nie,†a Zhimin Ao, *a Shaobin Wang b and Taicheng An a Author affiliations * Corresponding authors a Guangdong Key Laboratory of Environmental Catalysis and Health Risk Control, Guangzhou Key Laboratory of Environmental Catalysis and Pollution Control, School of Environmental Science and Engineering, Institute of Environmental Health and...
Recent progress in the g-C3N4 quantum dots: synthesis, properties and applications in photocatalytic degradation of organic pollutants
Recent progress in the g-C3N4 quantum dots: synthesis, properties and applications in photocatalytic degradation of organic pollutants Graphitic-carbon nitride quantum dots (g-C3N4QDs), as a rising star in the carbon nitride family, show great potentials in many fields involving bioimaging, fuel cells, and photo(electro)catalysis, endowed by their fascinating optical and electronic properties.
Correction: MXene as a non-metal charge mediator in 2D layered CdS@Ti3C2@TiO2 composites with superior Z-scheme visible light-driven photocatalytic activity
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MXene as non-metal charge mediator in 2D layered CdS@Ti3C2@TiO2 composites with superior Z-scheme visible light-driven photocatalytic activity
MXene as non-metal charge mediator in 2D layered CdS@Ti3C2@TiO2 composites with superior Z-scheme visible light-driven photocatalytic activity Qiaoran Liu, Xiaoyao Tan, Shaobin Wang, Fang Ma, Hussein Znad, Zhangfeng Shen, Lihong Liu and Shaomin Liu Abstract Exploitation of photocatalysts towards efficient organic pollutant degradation is highly desirable in the field of environmental remediation.
Photocatalytic conversion of lignocellulosic biomass to valuable products
Photocatalytic conversion of lignocellulosic biomass to valuable products Biomass is a naturally abundant, sustainable and clean resource, which has great potential to replace a portion of the finite petroleum and fossil feedstock for sustainable production of value-added chemicals and fuels. However, an efficient conversion process is still difficult to be achieved due to the complex nature of biomass.
Correction: AMPKα1 deletion shortens erythrocyte life span in mice: Role of oxidative stress.
See original article: Wang et al. 285 (26): 19976. VOLUME 285 (2010) PAGES 19976–19985 Supplemental Fig. 4 was mislabeled. This error has now been corrected and does not affect the results or conclusions of this work. The authors apologize for the error. © 2019 by The American Society for Biochemistry and Molecular Biology, Inc. Published in the U.S.A. The American Society for Biochemistry and Molecular Biology, Inc. Published in the U.S.A. Submit your work to JBC. You'll be in good company.
Histone Deacetylases (HDACs) Guided Novel Therapies for T-cell lymphomas
PDF Int J Med Sci 2019; 16(3):424-442. doi:10.7150/ijms.30154 Review Qing Zhang1 , Shaobin Wang2, Junhui Chen1, Zhendong Yu3 1. Department of Minimally Invasive Intervention, Peking University Shenzhen Hospital, Shenzhen, Guangdong, 518036, China. 2. Health Management Center of Peking University Shenzhen Hospital, Shenzhen, Guangdong, 518036, China. 3. China Central Laboratory of Peking University Shenzhen Hospital, Shenzhen, Guangdong, 518036, China.
Recent Advances in Transition Metal-Based Electrocatalysts for Alkaline Hydrogen Evolution
Recent Advances in Transition Metal-Based Electrocatalysts for Alkaline Hydrogen Evolution Zhijie Chen, Xiaoguang Duan, Wei Wei, Shaobin Wang and Bing-Jie Ni Abstract With the increasing demands in energy consumption and raising environmental concerns, it is of vital significance for developing renewable and clean energy sources to substitute traditional fossil fuels.
A Comparative Study of Metal (Ni, Co, or Mn)-Borate Catalysts and Their Photodeposition on rGO/ZnO Nanoarrays for Photoelectrochemical Water Splitting
Feasible and efficient photoelectrochemical (PEC) water splitting demands a rational integration of solar light absorbers with active electrocatalysts. Herein, we first compare three amorphous metal-borates (M-Bi, M = Ni, Co, Mn) as low-cost electrocatalysts, among which Mn-Bi is proposed for the first time for fabrication of new PEC devices for oxygen evolution reaction (OER).
Metal-Free Carbocatalysis in Advanced Oxidation Reactions
Catalytic processes have remarkably boosted the rapid industrializations in chemical production, energy conversion, and environmental remediation. As one of the emerging applications of carbocatalysis, metal-free nanocarbons have demonstrated promise as catalysts for green remediation technologies to overcome the poor stability and undesirable metal leaching in metal-based advanced oxidation processes (AOPs).
Atomic-level design of CoOH+-hydroxyapatite@C catalysts for superfast degradation of organics via peroxymonosulfate activation
F. Song, H. Zhang, S. Wang, L. Liu, X. Tan and S. Liu, Chem. Commun., 2018, 54, 4919 DOI: 10.1039/C8CC00946E If you are not the author of this article and you wish to reproduce material from it in a third party non-RSC publication you must formally request permission using RightsLink. Go to our Instructions for using RightsLink page for details.
Heterostructured WO3@CoWO4 bilayer nanosheets for enhanced visible-light photo, electro and photoelectro-chemical oxidation of water
Herein, a facile interface-induced synthesis method is first established to newly fabricate two-dimensional (2D) bilayer nanosheets of WO3@CoWO4 as highly efficient catalysts for enhanced photo, electro and photoelectro-chemical oxygen evolution reactions (OERs). The heterostructure and the interfacial oxygen vacancy of WO3@CoWO4 reduce the energy barriers in OER.
Singlet oxygen formation on bio-inspired synthesis of hollow Ag@AgBr photocatalyst for microbial and chemical decontamination
S. Zhang, H. Zhang, S. Wang, L. Liu and S. Liu, Catal. Sci. Technol., 2017, Accepted Manuscript , DOI: 10.1039/C7CY01131H If you are not the author of this article and you wish to reproduce material from it in a third party non-RSC publication you must formally request permission using RightsLink. Go to our Instructions for using RightsLink page for details.
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